A considerable amount of delta-3 would reduce 2/rev shake but at a penalty: reduced rotor damping and control crossup.
Rotor damping arises from the lag; something that disturbs the airframe is resisted because the rotor lags and supplies a restoring moment about the CG. Delta-3 imposes a kind of aerodynamic spring between rotor and airframe, tying them more tightly together.
With a normal rotor, force/displacement has a 90º relationship; with delta-3, the rotor resonant frequency is higher than rotational speed because of the aerodynamic spring and displacement is less than 90º. When the stick is pushed forward, there will be some sideways tilt of the rotor with delta-3.
I’ve played with delta-3 using model rotors running in front of a fan. With a seesaw rotor, delta angle can be set by skewing the teeter axis. At angles near 45º, things start getting squirrelly; the rotor will sometimes get into a nutational mode like a wobbling top.
The A&S 18-A has a huge amount of delta-3; it looks to be about 30º because it is the mechanism by which collective is lowered following a jump. As the rotor slows and coning angle increases, pitch is automatically pulled as a result of the coupling. The resulting cross control is partly compensated by swash plate phasing but can only be exact at a fixed flight condition; at others, the control crossup creeps back in.
Delta-3 is great for tail rotors but I’m not so sure it’s the magic bullet for main rotors.
But to answer your original question, Rusty, the violent shakers are the result of inplane resonance being excited by the 2/rev aerodynamic input. A rigid rotor pylon will almost always bring the rotor inplane resonance down to the 2/rev input. The cure is a limber mast combined with the stiffest possible rotor inplane.
The attached photo shows what Bell had to do to solve 2/rev on one of the B-47 precursors. The production model had the rotor stiffened internally.